CA: Civil War - pretty damn good. I think I liked Winter Soldier better, just because of the spy elements and mystery... but Civil War is by far my favorite "Avengers" movie (i mean, come on, it's Avengers 2.5).
It has the BEST action sequence in any comic book movie, possibly any movie (the airport scene). Just in awe the entire time (and if you have a real IMAX in your area - go see it there. That entire scene was shot on IMAX film). Fight choreography/effects throughout the movie were top-notch, and like most Marvel films, had a good mix of drama and some light-heartedness.
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